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the optoelectronic properties of colloidal CdS/ZnO composite nanoparticles with a carboxylated hexadentate Schiff base.
A novel, hexadentate, Schiff base ligand, N,N’-bis-(2-hydroxy-3-methoxy-5-carboxybenzylidene)-thiourea (HU6), with high stability and better solubility in aqueous media than the widely used tri- and tetradentate ligands, was synthesized using a condensation reaction of sodium thiocyanate and 3-carboxybenzaldehyde. The reduction-oxidation (redox) properties of the HU6 Schiff base-capped CdS nanoparticles (HU6-CdS) were studied systematically by a combination of optical, electroluminescence, X-ray diffraction, transmission and scanning electron microscopy techniques. The maximum enhancement in the photoluminescence emission occurs at the stoichiometric composition of 1:1 Cd:Cu in the Cu2+/Cu+ redox state of the HU6-CdS nanoparticles. Tuning the HU6-CdS nanoparticles with varying amounts of Cu+ induced broadening of the emission. The addition of Zn, Co and Ni as dopants, however, has a more negative impact on the emission efficiency of the Cu2+/Cu+ redox state. The redox-controlled PL enhancement under direct and indirect band-gap excitation has been attributed to the different radiative and nonradiative decay processes of the Cu2+/Cu+ redox state. The covalently attached HU6 Schiff base may be envisaged as a useful ligand for
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