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letsgo4theditiontestsandquizzesfreedownloadCooperativity of the interaction between paramagnetic dansyl chloride and a carbon chain: evidence for the role of hydroxyl groups in ferromagnetic exchange.
A study is reported of the use of nitroxide spin labels and a carbon chain fragment as a model of magnetic exchange in ferromagnetic and diamagnetic transition metal ions. In the first part of the study the interactions between the spin label and the alkyl chain were examined as a function of temperature and nitroxide concentration. At low spin concentration, an interaction between the spin label and the chain is observed, which is not due to homologous modulation of the spin label and the chain, but the result of magnetic exchange between the spin label and the chain. The interaction between the spin label and the chain increases as the spin concentration of the spin label increases. This interaction is identical in character to that between paramagnetic metal ions and the chain, suggesting that it arises from the interaction between the spin label and a carbon chain containing atoms that are similar to those in the paramagnetic metal ions. The energy barrier for dissociation of the spin label from the chain is found to be around 5 kcal mol-1, indicating that such an interaction is unlikely to interfere with the axial ferromagnetic magnetization exchange coupling in transition metal ions. Using an appropriate spin label and chain fragment, the energy of the magnetic exchange interaction between the paramagnetic metal ions and a chain was determined. The energy of the interaction is the same as that determined for the ferromagnetic exchange interaction between ferrous ions and a carbon chain fragment. On the basis of the results obtained with the spin label and carbon chain, a model is developed that describes the exchange interaction between paramagnetic metals and the carbon chain as a result of the exchange of the valence electron density between both molecules. The model allows the paramagnetic metals to be a linear combination of different geometrically relevant molecular orbitals, and these same orbitals are used to describe the exchange between the paramagnetic metal ions and the carbon chain. The above observations are a step toward better understanding of the role of the valence electron density in ferromagnetic exchange and may provide a route to the synthesis of paramagnetic or

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